Original Article
Copyright ©2012 Baishideng Publishing Group Co., Limited. All rights reserved.
World J Gastroenterol. Nov 14, 2012; 18(42): 6076-6087
Published online Nov 14, 2012. doi: 10.3748/wjg.v18.i42.6076
Galactosylated chitosan/5-fluorouracil nanoparticles inhibit mouse hepatic cancer growth and its side effects
Ming-Rong Cheng, Qing Li, Tao Wan, Bing He, Jiang Han, Hou-Xiang Chen, Feng-Xiao Yang, Wei Wang, Hong-Zhi Xu, Tao Ye, Bing-Bing Zha
Ming-Rong Cheng, Jiang Han, Wei Wang, Department of General Surgery, Shanghai Pudong New Area Zhoupu Hospital, Shanghai 201318, China
Qing Li, Department of General Medicine, Pujiang Branch of Shanghai Fifth People’s Hospital, Shanghai 201112, China
Tao Wan, Hou-Xiang Chen, Feng-Xiao Yang, Biomedical Materials and Engineering Center, Wuhan University of Technology, Wuhan 430070, Hubei Province, China
Ming-Rong Cheng, Bing He, Hong-Zhi Xu, Tao Ye, Department of General Surgery, Shanghai Fifth People’s Hospital, Fudan University, Shanghai 200240, China
Bing-Bing Zha, Department of Endocrine, Shanghai Fifth People’s Hospital, Fudan University, Shanghai 200240, China
Author contributions: Cheng MR, Li Q and Wan T contributed equally to this work; Cheng MR and Wan T designed the research; He B, Han J, Chen HX, Yang XF and Wang W performed the research; Xu HZ, Ye T and Zha BB analyzed the data; Cheng MR, Li Q and Wan T wrote the manuscript; and Cheng MR and Wan T revised the manuscript.
Supported by Natural Science Foundation of Shanghai, No. 09ZR1424700 and 114119a4700; Minhang District Natural Science Foundation of Shanghai, No. 2009MHZ085; and grants from Minhang District Public Health Bureau of Shanghai, No. 2009MW28
Correspondence to: Tao Wan, Associate Professor, Biomedical Materials and Engineering Center, Wuhan University of Technology, 122 Luoshi Road, Wuhan 430070, Hubei Province, China. wantao@whut.edu.cn
Telephone: +86-27-87651852 Fax: +86-27-87880734
Received: April 7, 2012
Revised: July 18, 2012
Accepted: July 28, 2012
Published online: November 14, 2012
Abstract

AIM: To observe the curative effect of galactosylated chitosan (GC)/5-fluorouracil (5-FU) nanoparticles in liver caner mice and its side effects.

METHODS: The GC/5-FU nanoparticle is a nanomaterial made by coupling GC and 5-FU. The release experiment was performed in vitro. The orthotropic liver cancer mouse models were established and divided into control, GC, 5-FU and GC/5-FU groups. Mice in the control and GC group received an intravenous injection of 200 μL saline and GC, respectively. Mice in the 5-FU and GC/5-FU groups received 200 μL (containing 0.371 mg 5-FU) 5-FU and GC/5-FU, respectively. The tumor weight and survival time were observed. The cell cycle and apoptosis in tumor tissues were monitored by flow cytometry. The expression of p53, Bax, Bcl-2, caspase-3 and poly adenosine 50-diphosphate-ribose polymerase 1 (PARP-1) was detected by immunohistochemistry, reverse transcription-polymerase chain reaction and Western blot. The serum blood biochemical parameters and cytotoxic activity of natural killer (NK) cell and cytotoxicity T lymphocyte (CTL) were measured.

RESULTS: The GC/5-FU nanoparticle is a sustained release system. The drug loading was 6.12% ± 1.36%, the encapsulation efficiency was 81.82% ± 5.32%, and the Zeta potential was 10.34 ± 1.43 mV. The tumor weight in the GC/5-FU group (0.4361 ± 0.1153 g vs 1.5801 ± 0.2821 g, P < 0.001) and the 5-FU (0.7932 ± 0.1283 g vs 1.5801 ± 0.2821 g, P < 0.001) was significantly lower than that in the control group; GC/5-FU treatment can significantly lower the tumor weight (0.4361 ± 0.1153 g vs 0.7932 ± 0.1283 g, P < 0.001), and the longest median survival time was seen in the GC/5-FU group, compared with the control (12 d vs 30 d, P < 0.001), GC (13 d vs 30 d, P < 0.001) and 5-FU groups (17 d vs 30 d, P < 0.001). Flow cytometry revealed that compared with the control, GC/5-FU caused a higher rate of G0-G1 arrest (52.79% ± 13.42% vs 23.92% ± 9.09%, P = 0.014 ) and apoptosis (2.55% ± 1.10% vs 11.13% ± 11.73%, P < 0.001) in hepatic cancer cells. Analysis of the apoptosis pathways showed that GC/5-FU upregulated the expression of p53 at both the protein and the mRNA levels, which in turn lowered the ratio of Bcl-2/Bax expression; this led to the release of cytochrome C into the cytosol from the mitochondria and the subsequent activation of caspase-3. Upregulation of caspase-3 expression decreased the PARP-1 at both the mRNA and the protein levels, which contributed to apoptosis. 5-FU increased the levels of aspartate aminotransferase and alanine aminotransferase, and decreased the numbers of platelet, white blood cell and lymphocyte and cytotoxic activities of CTL and NK cells, however, there were no such side effects in the GC/5-FU group.

CONCLUSION: GC/5-FU nanoparticles can significantly inhibit the growth of liver cancer in mice via the p53 apoptosis pathway, and relieve the side effects and immunosuppression of 5-FU.

Keywords: Galactosylated chitosan; Nanoparticles; 5-fluorouracil; Hepatocellular cancer; Targeted therapy; Apoptosis